Tooru Kirishima's notoriety is spread far and wide in the underworld. He is most commonly known as "The Demon of Sakuragi"—a man who is not afraid to resort to violence if deemed necessary. After almost jeopardizing a peace treaty, his boss tasks him with the most difficult job he has ever had: taking care of seven-year-old Yaeka Sakuragi—the boss' precious daughter—so that Tooru understands what it means to be responsible for another life. At first, the two do not seem to meet eye to eye, as Tooru has no clue on how to communicate with Yaeka, and the young girl is not used to expressing her emotions. However, as time goes on, they come to understand each other despite their differences. The fearsome right-hand man of a yakuza boss and the child he must protect are about to learn that family is not always bound by blood.

Hot on the heels of the third year students' graduation, μ's is invited to New York in hopes of spreading the joy of school idols to other parts of the world. Due to the events of the recent Love Live!, μ's has reached eminent stardom which results in crowds swarming them whenever they appear in public. With the increased attention, however, comes a difficult choice. Having yet to publicly announce the decision they came to regarding their future, the young members of μ's are pushed to continue performing by rival group A-RISE, Otonokizaka High School, and even Love Live! itself. As leader, Honoka Kousaka is left wondering if the path they have chosen is truly for the best, as μ's must re-evaluate their choices and come to a final decision on what they want for the future. Love Live! The School Idol Movie depicts the final chapter in μ's story as the girls explore just what being an idol means to them as well as the bond that connects the nine of them together.

In the distant future, a majority of humans have left the Earth, and the Galactic Alliance of Humanity is founded to guide exploration and ensure the prosperity of mankind. However, a significant threat arises in the form of strange creatures called Hideauze, resulting in an interstellar war to prevent humanity's extinction. Armed with Chamber, an autonomous robot, 16-year-old lieutenant Ledo of the Galactic Alliance joins the battle against the monsters. In an unfortunate turn of events, Ledo loses control during the battle and is cast out to the far reaches of space, crash-landing on a waterlogged Earth. On the blue planet, Gargantia—a large fleet of scavenger ships—comes across Chamber and retrieves it from the ocean, thinking they have salvaged something of value. Mistaking their actions for hostility, Ledo sneaks aboard and takes a young messenger girl named Amy hostage, only to realize that the residents of Gargantia are not as dangerous as he had believed. Faced with uncertainty, and unable to communicate with his comrades in space, Ledo attempts to get his bearings and acclimate to a new lifestyle. But his peaceful days are about to be short-lived, as there is more to this ocean-covered planet than meets the eye.

A special episode focusing on the story of Merm4id and Rondo, including a new, joint performance by the two groups.